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Chichester Cathedral – a magnificent building with beautiful Marc Chagall stained glass window, nice refectory behind for lunch/coffee & Bishops Garden (also behind) is pretty walled garden.
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Fishbourne Roman Palace – fantastic Roman mosaic floors etc
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West Wittering Beach – great beach for walks & swims,
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Goodwood Sculpture Park – about £10 to get in but well worth a visit
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Pallant House Gallery in Chichester – new wing housing contempory collection that recently won Gulbenkian prize.
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West Dean Gardens – beautiful Victorian walled garden
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Weald & Downland Musem – next to West Dean, old farm buildings from various periods, nicely laid out to walk around.
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Arundel – about 20 min. drive away but it's got the Castle, lots of antiques, nice restaurants
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Uppark House – National Trust stately home
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Portsmouth Ancient Dockyard – Mary Rose, Victory etc
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Spinnaker Tower – Gunwharf Quay, a great landmark & fun to go up on a clear day.